Hey, I'm the one who did the research on New Albion Ale. I just noticed this thread!
I don't have any information on the water beyond what is posted. But I have a few general thoughts on this:
1) As far as I know, English brewers harden their water much more than American brewers. Maybe Martin can tell us if I'm off-base on that. Given that a lot of the homebrewing and available professional brewing knowledge in 1976 was of English provenance, it wouldn't be surprising to me that they were truly hardening the water to Barley's recollection based on English practices.
2) Someone on reddit was disparaging New Albion as if they must have been bumpkins in terms of knowledge. I was able to respond with a quote from Jack McCauliffe to the effect that running New Albion was like three jobs: (a) studying at the library; (b) manufacturing and maintaining the brewery; and (c) brewing and distributing. I don't have the exact quote at hand. The point is that McCauliffe and Barkley were no rubes, were only 50 mi. away from the library at UC-Davis, and had access to the brains of the brewers at Anchor (not to mention some technical assistance from Coors). I am sure they had their water chemistry sorted out.
3) If anyone is skeptical. it would be easy to brew to a more 'modern' water profile and then dose some beer with gypsum to achieve the purported profile stated by Don Barkley. Or you could pick up the phone and call him.
Cheers,
Chino